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학술지 Nanoscale Biomemory Composed of Recombinant Azurin on a Nanogap Electrode
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저자
정용호, 이택, 박형주, 윤완수, 민준홍, 최정우
발행일
201309
출처
Nanotechnology, v.24 no.36, pp.1-8
ISSN
0957-4484
출판사
Institute of Physics (IOP)
DOI
https://dx.doi.org/10.1088/0957-4484/24/36/365301
초록
We fabricate a nanoscale biomemory device composed of recombinant azurin on nanogap electrodes. For this, size-controllable nanogap electrodes are fabricated by photolithography, electron beam lithography, and surface catalyzed chemical deposition. Moreover, we investigate the effect of gap distance to optimize the size of electrodes for a biomemory device and explore the mechanism of electron transfer from immobilized protein to a nanogap counter-electrode. As the distance of the nanogap electrode is decreased in the nanoscale, the absolute current intensity decreases according to the distance decrement between the electrodes due to direct electron transfer, in contrast with the diffusion phenomenon of a micro-electrode. The biomemory function is achieved on the optimized nanogap electrode. These results demonstrate that the fabricated nanodevice composed of a nanogap electrode and biomaterials provides various advantages such as quantitative control of signals and exclusion of environmental effects such as noise. The proposed bioelectronics device, which could be mass-produced easily, could be applied to construct a nanoscale bioelectronics system composed of a single biomolecule. © 2013 IOP Publishing Ltd.
KSP 제안 키워드
Chemical deposition, Current intensity, Direct electron transfer(eT), Environmental effects, Gap distance, Micro-electrode, Nano-gap electrode, Nanoscale biomemory, Quantitative control, Recombinant azurin, Size-controllable