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Journal Article Evaluation of Nonlinear Optical Polymers for Second-Harmonic Generation: Toward the Balance of Absorption and Nonlinearity Against Intrinsic Trade-Off
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Authors
Min Su Kim, Jung Jin Ju, Seung Koo Park, Jung Yun Do, Myung Hyun Lee
Issue Date
2006-01
Citation
Chemical Physics Letters, v.417, no.1-3, pp.277-281
ISSN
0009-2614
Publisher
Elsevier
Language
English
Type
Journal Article
DOI
https://dx.doi.org/10.1016/j.cplett.2005.10.034
Abstract
Despite many advantages toward nonlinear optical (NLO) waveguide devices, NLO polymers have not been adopted successfully into practical wavelength converters due to their high absorption losses. Empirical and theoretical understandings about NLO susceptibility imply the fundamental trade-off between optical absorption and nonlinearity. Our theoretical analysis elucidates the effect of absorption losses on second-harmonic generation (SHG). We compare analytically maximum conversion efficiencies for several NLO polymers and found a convincing approach for the development of NLO polymers with the optimum combination of high optical nonlinearity and low material absorption, which leads us to realize efficient polymeric SHG devices. © 2005 Elsevier B.V. All rights reserved.
KSP Keywords
Conversion efficiency(C.E.), High absorption, Material absorption, Nonlinear optical polymers, Optical absorption, Optical nonlinearity, Second Harmonic Generation, Theoretical Analysis, Trade-off, waveguide device, wavelength converter