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Journal Article
Mott Switching and Structural Transition in the Metal Phase of VO2 Nanodomain
- Authors
- Chang-Yong Kim, Tetiana Slusar, Jinchul Cho, Hyun-Tak Kim
- Issue Date
- 2021-02
- Citation
- ACS Applied Electronic Materials, v.3, no.2, pp.605-610
- ISSN
- 2637-6113
- Publisher
- American Chemical Society(ACS)
- Language
- English
- Type
- Journal Article
- Abstract
- VO2 undergoes the insulator-metal transition (IMT) and monoclinic-rutile structural phase transition (SPT) near 67 °C. The IMT switching has many applications. However, there is an unresolved issue whether the IMT is a Mott transition or a Peierls transition. This complication is caused by metal and insulator coexistence, which is an inherent property of the IMT region. Thus, the acquired data in the IMT region are averaged over the two phases in many experiments. We overcome the issue by probing the electronic state of the monoclinic structure and by introducing a model that accounts for the coexisting phases. We reveal the Mott IMT in the nondistorted monoclinic nanodomain between 55 and 63 °C and the distortion-assisted SPT above 60 °C.
- KSP Keywords
- Electronic state, Metal phase, Mott transition, Two-phase, insulator-metal transition, monoclinic structure, peierls transition, structural phase transition, structural transition
This work is distributed under the term of Creative Commons License (CCL)
(CC BY NC ND)
(CC BY NC ND)
