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Journal Article Growth Behaviors of InAs/GaAs Quantum Dots Using Metal−Organic Chemical Vapor Deposition with Dual-Channel AsH3 Supply and H2 Carrier Gas Flow Rate Variation
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Authors
HoSung Kim, Mireu Lee, Dae-Myeong Geum, Young-Ho Ko
Issue Date
2025-08
Citation
Crystal Growth and Design, v.25, no.16, pp.6628-6635
ISSN
1528-7483
Publisher
American Chemical Society
Language
English
Type
Journal Article
DOI
https://dx.doi.org/10.1021/acs.cgd.5c00547
Abstract
In this study, we conducted a comprehensive investigation into the effects of a dual-channel arsine (AsH3) supply and varying hydrogen (H2) carrier gas flow rates on the growth of InAs/GaAs quantum dots (QDs) via metal–organic vapor deposition (MOCVD). The implementation of a dual-channel AsH3 supply resulted in more stable and uniform QD growth compared with the conventional single-channel configuration, primarily due to the abrupt change in the V/III ratio. Moreover, the H2 flow rate was found to play a critical role in determining the QD size distribution and optical performance. Notably, at a moderate H2 flow rate of 100 sccm, enhanced QD size uniformity and increased photoluminescence (PL) intensity were observed. These findings provide valuable insights into achieving high-quality InAs/GaAs QDs through precise control of the AsH3 supply configuration and H2 carrier gas flow during the MOCVD growth process.